Some of this I've used in other formats and some I just found.
Old School: You can't go wrong with Don Schowalter. World of Chemistry. I still have the VHS tapes. Timeless. Here is the link you can stream and a link for worksheets that I found.
http://www.learner.org/resources/series61.html?pop=yes&pid=793#
http://www.hschem.org/Resources/worldofchemistry/worldofchemistry.htm
Here are some sims from Iowa State. I've never used these but I tried and couple and they look good.
Chemistry Experiment Simulations and Conceptual Computer Animations
http://www.chem.iastate.edu/group/Greenbowe/sections/projectfolder/simDownload/index4.html#thermoChem
I have the disc for Chemistry Comes Alive! It's a good series of video and stills from ACS. You can download it for free from itunes. I don't if it's the entire series or pieces.
http://itunes.apple.com/us/itunes-u/chemistry-comes-alive-videos/id391599380
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